Caribe Tours leave from Santiago to go to Dajabon, which would require you first going there, then transferring.
If that is your only option, the busses leave Puerto Plata for Santiago at 6:00 7:00 8:00 9:00 10:00 11:00 12:00 AM & 1:00 2:00 3:00 4:00 5:00 6:00 7:00 PM, then you would allow approx. 1 hour to arrive in Santiago, then the busses leave for Dajabon at 9:00 10:30 AM 12 noon & 3:30 4:30 6:00 PM
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