Cayo Levantado is an island in the Bay of Samana. There are boats going back and forth from the pier in Samana. Jarabacoa is in the mountain area in central part of country. If it isn't shown on your map, look for La Vega. It is in that general area.
There is a Caribe Tour bus to Samana that leaves Puerto Plata at 7am and Sosua at 7:30. Gets to Samana about 10:45. Leaves Samana at 4pm. You would be very, very pressed for time to go to Cayo Levantado the same day, but it could be done. Better to spend the night in Samana.
Getting to Jarabacoa also possible by bus, but some bus changing will be necessary enroute. It is definitely not a day trip.
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