Metro bús used to have a station in Moca, but that service was discontinued a couple of years ago.
In terms of travel time, Moca is 30 minutes to either Santiago or Salcedo. The road between Moca and Salcedo is not that bad, there are a few stretches where it gets bumpy; but for the most part its a good road. The same is true between Santiago and Moca.
Its really your pick, STG or SLD. Eitherway, you will be a half hour or so from Moca.
-NALS
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